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Yuan, F., Folpini, G., Liu, T., Singh, U., Treglia, A., Lim, J. W., . . . Gao, F. (2024). Bright and stable near-infrared lead-free perovskite light-emitting diodes. Nature Photonics, 18, 170-176
Open this publication in new window or tab >>Bright and stable near-infrared lead-free perovskite light-emitting diodes
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2024 (English)In: Nature Photonics, ISSN 1749-4885, E-ISSN 1749-4893, Vol. 18, p. 170-176Article in journal (Refereed) Published
Abstract [en]

Long-wavelength near-infrared light-emitting diodes (NIR LEDs) with peak emission wavelengths beyond 900 nm are of critical importance for various applications including night vision, biomedical imaging, sensing and optical communications. However, the low radiance and poor operational stability of state-of-the-art long-wavelength NIR LEDs based on soft materials remain the most critical factors limiting their practical applications. Here we develop NIR LEDs emitting beyond 900 nm with improved performance through the rational manipulation of p doping in all-inorganic tin perovskites (CsSnI3) by retarding and controlling the crystallization process of perovskite precursors in tin-rich conditions. The resulting NIR LEDs exhibit a peak emission wavelength at 948 nm, high radiance of 226 W sr-1 m-2 and long operational half-lifetime of 39.5 h at a high constant current density of 100 mA cm-2. Our demonstration of efficient and stable NIR LEDs operating at high current densities may also open up new opportunities towards electrically pumped lasers. Controlling the intrinsic doping of lead-free perovskites enables near-infrared LEDs emitting at 948 nm with a peak radiance of 226 W sr-1 m-2 and a half-lifetime of 39.5 h.

Place, publisher, year, edition, pages
NATURE PORTFOLIO, 2024
National Category
Atom and Molecular Physics and Optics
Identifiers
urn:nbn:se:liu:diva-200236 (URN)10.1038/s41566-023-01351-5 (DOI)001137092700001 ()
Note

Funding Agencies|National Key Research and Development Program of China; National Natural Science Foundation of China; National Science Fund for Excellent Young Scholars (Overseas) and Special Funds for Introducing Talents from Beijing Normal University; Knut and Alice Wallenberg Foundation; European Research Council; Swedish Research Council Vetenskapsradet; Swedish Government Strategic Research Area in Materials Science on Functional Materials at Linkoeping University (faculty grant SFO-Mat-LiU); Wallenberg Academy [2023YFB3611800]; Swedish Research Council (VR) [22302012]; ERC [312200502508]; Singapore Ministry of Education under its MOE Tier 2 grant [KAW 2019.0082]; National Research Foundation (NRF) Singapore under its NRF Investigatorship [101045098]; European Union's Horizon 2020 research and innovation programme through the ERC project SOPHY [2020-03564]; MSCA-ITN SMART-X [2009-00971]; Marie Sklodowska-Curie grant [KAW-2018.0194]; Swedish Research Council [2019-05551]; [854843]; [MOE-T2EP50120-0004]; [NRF-NRFI2018-04]; [771528]; [860553]; [956270]; [2022-06725]; [2018-05973]

Available from: 2024-01-18 Created: 2024-01-18 Last updated: 2024-11-22Bibliographically approved
Ji, F., Klarbring, J., Zhang, B., Wang, F., Wang, L., Miao, X., . . . Gao, F. (2024). Remarkable Thermochromism in the Double Perovskite Cs2NaFeCl6. Advanced Optical Materials, 12(8), Article ID 2301102.
Open this publication in new window or tab >>Remarkable Thermochromism in the Double Perovskite Cs2NaFeCl6
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2024 (English)In: Advanced Optical Materials, ISSN 2162-7568, E-ISSN 2195-1071, Vol. 12, no 8, article id 2301102Article in journal (Refereed) Published
Abstract [en]

Lead-free halide double perovskites (HDPs) have emerged as a new generation of thermochromic materials. However, further materials development and mechanistic understanding are required. Here, a highly stable HDP Cs2NaFeCl6 single crystal is synthesized, and its remarkable and fully reversible thermochromism with a wide color variation from light-yellow to black over a temperature range of 10 to 423 K is investigated. First-principles, density functional theory (DFT)-based calculations indicate that the thermochromism in Cs2NaFeCl6 is an effect of electron–phonon coupling. The temperature sensitivity of the bandgap in Cs2NaFeCl6 is up to 2.52 meVK−1 based on the Varshni equation, which is significantly higher than that of lead halide perovskites and many conventional group-IV, III–V semiconductors. Meanwhile, this material shows excellent environmental, thermal, and thermochromic cycle stability. This work provides valuable insights into HDPs' thermochromism and sheds new light on developing efficient thermochromic materials.

Place, publisher, year, edition, pages
Wiley-Blackwell, 2024
National Category
Physical Chemistry
Identifiers
urn:nbn:se:liu:diva-197177 (URN)10.1002/adom.202301102 (DOI)001049682400001 ()2-s2.0-85168260340 (Scopus ID)
Funder
Knut and Alice Wallenberg Foundation, Dnr. KAW 2019.0082Swedish Energy Agency, 2018‐004357Swedish Research Council, 2021‐00357Swedish Research Council, 2019–05551Swedish Research Council, 2022–06725Swedish Research Council, 2018–05973
Note

Funding agencies: This work was financially supported by the Knut and Alice Wallenberg Foundation (Dnr. KAW 2019.0082), the Swedish Energy Agency (2018-004357), Carl Tryggers Stiftelse, Olle Engkvist Byggmästare Stiftelse, and the Swedish Government Strategic Research Area in Materials Science on Functional Materials at Linköping University (Faculty Grant SFO-Mat-LiU No. 2009-00971). I.A.A. is a Wallenberg Scholar. B.B. gratefully acknowledges financial support from the Swedish Research Council (VR) grant no. 2021-00357. F.J. was supported by the China Scholarship Council (CSC). W.N. acknowledges the Suzhou Key Laboratory of Functional Nano & Soft Materials, the Collaborative Innovation Center of Suzhou Nano Science & Technology (NANO−CIC), and the 111 Project for the financial support. S.I.S. acknowledges the support from the Swedish Research Council (VR) (Project No. 2019–05551) and the ERC (synergy grant FASTCORR project 854843). The computations were enabled by resources provided by the National Academic Infrastructure for Supercomputing in Sweden (NAISS), the Swedish National Infrastructure for Computing (SNIC) at the National Supercomputer Center (NSC), and the Center for High Performance Computing (PDC), partially funded by the Swedish Research Council through Grant Agreements No. 2022–06725 and No. 2018–05973. F.W. gratefully acknowledges financial support from the Open Project Funding of Jiangsu Key Laboratory for Carbon-based Functional Materials & Devices, Soochow University (KJS2152), and the Formas (2020-03001). M.M. acknowledges financial support from Swedish Energy Research (Grant no. 43606-1) and the Carl Tryggers Foundation (CTS20:272, CTS16:303, CTS14:310).

Available from: 2023-08-24 Created: 2023-08-24 Last updated: 2025-02-14Bibliographically approved
Knoop, F., Shulumba, N., Castellano, A., Alvarinhas Batista, J., Farris, R., Verstraete, M. J., . . . Hellman, O. (2024). TDEP:Temperature Dependent Effective Potentials. Journal of Open Source Software, 9(94), Article ID 6150.
Open this publication in new window or tab >>TDEP:Temperature Dependent Effective Potentials
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2024 (English)In: Journal of Open Source Software, E-ISSN 2475-9066, Vol. 9, no 94, article id 6150Article in journal (Refereed) Published
Abstract [en]

The Temperature Dependent Effective Potential (TDEP) method is a versatile and efficient approach to include temperature in a binitio materials simulations based on phonon theory. TDEP can be used to describe thermodynamic properties in classical and quantum ensembles, and several response properties ranging from thermal transport to Neutron and Raman spectroscopy. A stable and fast reference implementation is given in the software package of the same name described here. The underlying theoretical framework and foundation is briefly sketched with an emphasis on discerning the conceptual difference between bare and effective phonon theory, in both self-consistent and non-self-consistent formulations. References to numerous applications and more in-depth discussions of the theory are given.

Place, publisher, year, edition, pages
Open journals, 2024
National Category
Condensed Matter Physics
Identifiers
urn:nbn:se:liu:diva-200749 (URN)10.21105/joss.06150 (DOI)
Available from: 2024-02-08 Created: 2024-02-08 Last updated: 2024-02-08
Mopoung, K., Ning, W., Zhang, M., Ji, F., Mukhuti, K., Engelkamp, H., . . . Puttisong, Y. (2024). Understanding Antiferromagnetic Coupling in Lead-Free Halide Double Perovskite Semiconductors. The Journal of Physical Chemistry C, 128(12), 5313-5320
Open this publication in new window or tab >>Understanding Antiferromagnetic Coupling in Lead-Free Halide Double Perovskite Semiconductors
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2024 (English)In: The Journal of Physical Chemistry C, ISSN 1932-7447, E-ISSN 1932-7455, Vol. 128, no 12, p. 5313-5320Article in journal (Refereed) Published
Abstract [en]

Solution-processable semiconductors with antiferromagnetic (AFM) order are attractive for future spintronics and information storage technology. Halide perovskites containing magnetic ions have emerged as multifunctional materials, demonstrating a cross-link between structural, optical, electrical, and magnetic properties. However, stable optoelectronic halide perovskites that are antiferromagnetic remain sparse, and the critical design rules to optimize magnetic coupling still must be developed. Here, we combine the complementary magnetometry and electron-spin-resonance experiments, together with first-principles calculations to study the antiferromagnetic coupling in stable Cs-2(Ag:Na)FeCl6 bulk semiconductor alloys grown by the hydrothermal method. We show the importance of nonmagnetic monovalence ions at the B-I site (Na/Ag) in facilitating the superexchange interaction via orbital hybridization, offering the tunability of the Curie-Weiss parameters between -27 and -210 K, with a potential to promote magnetic frustration via alloying the nonmagnetic B-I site (Ag:Na ratio). Combining our experimental evidence with first-principles calculations, we draw a cohesive picture of the material design for B-site-ordered antiferromagnetic halide double perovskites.

Place, publisher, year, edition, pages
AMER CHEMICAL SOC, 2024
National Category
Condensed Matter Physics
Identifiers
urn:nbn:se:liu:diva-202270 (URN)10.1021/acs.jpcc.3c08129 (DOI)001185377800001 ()38567374 (PubMedID)
Note

Funding Agencies|Energimyndigheten [2022-06725, 2018-05973]; Swedish Research Council [KAW 2019.0082]; Knut and Alice Wallenberg Foundation [Dnr 48758-1, Dnr 48594-1]; Swedish Energy Agency [2009-00971]; Swedish Government Strategic Research Area in Materials Science on Functional Materials at Linkoping University [CTS 20:350]; Carl-Trygger Foundation [2023-05247]; Swedish Research Council (VR) [854843]; ERC [KAW-2018.0194]; Wallenberg Academy Scholar

Available from: 2024-04-09 Created: 2024-04-09 Last updated: 2025-02-14
Pilemalm, R., Simak, S. & Eklund, P. (2019). The Effect of Point Defects on the Electronic Density of States of ScMN2-Type (M = V, Nb, Ta) Phases. Condensed Matter, 4(3), Article ID 70.
Open this publication in new window or tab >>The Effect of Point Defects on the Electronic Density of States of ScMN2-Type (M = V, Nb, Ta) Phases
2019 (English)In: Condensed Matter, ISSN 2410-3896, Vol. 4, no 3, article id 70Article in journal (Refereed) Published
Abstract [en]

ScMN2-type (M = V, Nb, Ta) phases are layered materials that have been experimentally reported for M = Ta and Nb. They are narrow-bandgap semiconductors with potentially interesting thermoelectric properties. Point defects such as dopants and vacancies largely affect these properties, motivating the need to investigate these effects. In particular, asymmetric peak features in the density of states (DOS) close to the highest occupied state is expected to increase the Seebeck coefficient. Here, we used first principles calculations to study the effects of one vacancy or one C, O, or F dopant on the DOS of the ScMN2 phases. We used density functional theory to calculate formation energy and the density of states when a point defect is introduced in the structures. In the DOS, asymmetric peak features close to the highest occupied state were found as a result of having a vacancy in all three phases. Furthermore, one C dopant in ScTaN2, ScNbN2, and ScVN2 implies a shift of the highest occupied state into the valence band, while one O or F dopant causes a shift of the highest occupied state into the conduction band.

Place, publisher, year, edition, pages
MDPI, 2019
Keywords
ScTaN2; YNbN2; inverse MAX phase; point defect; density of states
National Category
Physical Sciences
Identifiers
urn:nbn:se:liu:diva-160948 (URN)10.3390/condmat4030070 (DOI)000487966200001 ()
Note

Funding agencies: Swedish Research Council (VR)Swedish Research Council [2016-03365]; Knut and Alice Wallenberg Foundation through the Wallenberg Academy Fellows program; Swedish Government Strategic Research Area in Materials Science on Functional Materials at Linkoping U

Available from: 2019-10-16 Created: 2019-10-16 Last updated: 2019-11-04Bibliographically approved
Pilemalm, R., Pourovskii, L., Mosyagin, I., Simak, S. & Eklund, P. (2019). Thermodynamic Stability, Thermoelectric, Elastic and Electronic Structure Properties of ScMN2-Type (M = V, Nb, Ta) Phases Studied by ab initio Calculations. Condensed Matter, 4(2), Article ID 36.
Open this publication in new window or tab >>Thermodynamic Stability, Thermoelectric, Elastic and Electronic Structure Properties of ScMN2-Type (M = V, Nb, Ta) Phases Studied by ab initio Calculations
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2019 (English)In: Condensed Matter, ISSN 2410-3896, Vol. 4, no 2, article id 36Article in journal (Refereed) Published
Abstract [en]

ScMN2-type (M = V, Nb, Ta) phases are layered materials that have been experimentally reported for M = Ta and Nb, but they have up to now not been much studied. However, based on the properties of binary ScN and its alloys, it is reasonable to expect these phases to be of relevance in a range of applications, including thermoelectrics. Here, we have used first-principles calculations to study their thermodynamic stability, elastic, thermoelectric and electronic properties. We have used density functional theory to calculate lattice parameters, the mixing enthalpy of formation and electronic density of states as well as the thermoelectric properties and elastic constants (cij), bulk (B), shear (G) and Young’s (E) modulus, which were compared with available experimental data. Our results indicate that the considered systems are thermodynamically and elastically stable and that all are semiconductors with small band gaps. All three materials display anisotropic thermoelectric properties and indicate the possibility to tune these properties by doping. In particular, ScVN2, featuring the largest band gap exhibits a particularly large and strongly doping-sensitive Seebeck coefficient.

Place, publisher, year, edition, pages
Basel: MDPI, 2019
Keywords
ScTaN2; inverse MAX phase; thermoelectric properties; density functional theory
National Category
Physical Sciences Condensed Matter Physics
Identifiers
urn:nbn:se:liu:diva-156671 (URN)10.3390/condmat4020036 (DOI)000475286700002 ()
Note

Funding agencies: Swedish Research Council (VR) [2016-03365]; Knut and AliceWallenberg Foundation through the Academy Fellows Program; Swedish Government Strategic Research Area in Materials Science on Functional Materials at Linkoping University [2009 00971]; European Res

Available from: 2019-05-07 Created: 2019-05-07 Last updated: 2019-07-30Bibliographically approved
Burakovsky, L., Burakovsky, N., Preston, D. & Simak, S. I. (2018). Systematics of the Third Row Transition Metal Melting: The HCP Metals Rhenium and Osmium. Crystals, 8(6), Article ID 243.
Open this publication in new window or tab >>Systematics of the Third Row Transition Metal Melting: The HCP Metals Rhenium and Osmium
2018 (English)In: Crystals, ISSN 2073-4352, Vol. 8, no 6, article id 243Article in journal (Refereed) Published
Abstract [en]

The melting curves of rhenium and osmium to megabar pressures are obtained from an extensive suite of ab initio quantum molecular dynamics (QMD) simulations using the Z method. In addition, for Re, we combine QMD simulations with total free energy calculations to obtain its phase diagram. Our results indicate that Re, which generally assumes a hexagonal close-packed (hcp) structure, melts from a face-centered cubic (fcc) structure in the pressure range 20-240 GPa. We conclude that the recent DAC data on Re to 50 GPa in fact encompass both the true melting curve and the low-slope hcp-fcc phase boundary above a triple point at (20 GPa, 4240 K). A linear fit to the Re diamond anvil cell (DAC) data then results in a slope that is 2.3 times smaller than that of the actual melting curve. The phase diagram of Re is topologically equivalent to that of Pt calculated by us earlier on. Regularities in the melting curves of Re, Os, and five other 3rd-row transition metals (Ta, W, Ir, Pt, Au) form the 3rd-row transition metal melting systematics. We demonstrate how this systematics can be used to estimate the currently unknown melting curve of the eighth 3rd-row transition metal Hf.

Place, publisher, year, edition, pages
MDPI, 2018
Keywords
quantum molecular dynamics; phase diagram; melting curve; transition metal
National Category
Condensed Matter Physics
Identifiers
urn:nbn:se:liu:diva-149722 (URN)10.3390/cryst8060243 (DOI)000436129400012 ()
Note

Funding Agencies|US DOE/NNSA

Available from: 2018-07-24 Created: 2018-07-24 Last updated: 2018-08-14
Kerdsongpanya, S., Hellman, O., Sun, B., Kan Koh, Y., Lu, J., Van Nong, N., . . . Eklund, P. (2017). Phonon thermal conductivity of scandium nitride for thermoelectrics from first-principles calculations and thin-film growth. Physical Review B, 96(19), Article ID 195417.
Open this publication in new window or tab >>Phonon thermal conductivity of scandium nitride for thermoelectrics from first-principles calculations and thin-film growth
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2017 (English)In: Physical Review B, ISSN 2469-9950, E-ISSN 2469-9969, Vol. 96, no 19, article id 195417Article in journal (Refereed) Published
Abstract [en]

The knowledge of lattice thermal conductivity of materials under realistic conditions is vitally important since many modern technologies require either high or low thermal conductivity. Here, we propose a theoretical model for determining lattice thermal conductivity, which takes into account the effect of microstructure. It is based on ab initio description that includes the temperature dependence of the interatomic force constants and treats anharmonic lattice vibrations. We choose ScN as a model system, comparing the computational predictions to the experimental data by time-domain thermoreflectance. Our experimental results show a trend of reduction in lattice thermal conductivity with decreasing domain size predicted by the theoretical model. These results suggest a possibility to control thermal conductivity by microstructural tailoring and provide a predictive tool for the effect of the microstructure on the lattice thermal conductivity of materials based on ab initio calculations.

Place, publisher, year, edition, pages
American Physical Society, 2017
National Category
Condensed Matter Physics
Identifiers
urn:nbn:se:liu:diva-143238 (URN)10.1103/PhysRevB.96.195417 (DOI)000414738200008 ()
Note

Funding Agencies|European Research Council under the European Communitys Seventh Framework Programme [FP/2007-2013]; ERC [335383]; Swedish Government Strategic Research Area in Materials Science on Functional Materials at Linkoping University [2009 00971]; Swedish Research Council [2012-4430, 2016-03365, 330-2014-6336, 2014-4750, 637-2013-7296]; Linnaeus Environment LiLi-NFM; Swedish Foundation for Strategic Research (SSF) through the Future Research Leaders 5 Program; NanoCaTe project (FP7) [604647]; National University of Singapore Startup Grant

Available from: 2017-11-27 Created: 2017-11-27 Last updated: 2017-12-05Bibliographically approved
Wang, F., Abrikosov, I., Simak, S., Odén, M., Muecklich, F. & Tasnadi, F. (2016). Coherency effects on the mixing thermodynamics of cubic Ti1-xAlxN/TiN(001) multilayers. PHYSICAL REVIEW B, 93(17), 174201
Open this publication in new window or tab >>Coherency effects on the mixing thermodynamics of cubic Ti1-xAlxN/TiN(001) multilayers
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2016 (English)In: PHYSICAL REVIEW B, ISSN 2469-9950, Vol. 93, no 17, p. 174201-Article in journal (Refereed) Published
Abstract [en]

In this work, we discuss the mixing thermodynamics of cubic (B1) Ti1-xAlxN/TiN(001) multilayers. We show that interfacial effects suppress the mixing enthalpy compared to bulk Ti1-xAlxN. The strongest stabilization occurs for compositions in which the mixing enthalpy of bulk Ti1-xAlxN has its maximum. The effect is split into a strain and an interfacial (or chemical) contribution, and we show that both contributions are significant. An analysis of the local atomic structure reveals that the Ti atoms located in the interfacial layers relax significantly different from those in the other atomic layers of the multilayer. Considering the electronic structure of the studied system, we demonstrate that the lower Ti-site projected density of states at epsilon(F) in the Ti1-xAlxN/TiN multilayers compared to the corresponding monolithic bulk explains a decreased tendency toward decomposition.

Place, publisher, year, edition, pages
AMER PHYSICAL SOC, 2016
National Category
Condensed Matter Physics
Identifiers
urn:nbn:se:liu:diva-129166 (URN)10.1103/PhysRevB.93.174201 (DOI)000375990200003 ()
Note

Funding Agencies|Swedish Foundation for Strategic Research (SSF) project SRL [10-0026]; Erasmus Mundus Joint European Doctoral Programme DocMASE; Multiscale computational-design of novel hard nanostructure coatings; Swedish Research Council (VR) [2015-04391, 621-2012-4401, 2014-4750]; Grant of Ministry of Education and Science of the Russian Federation [14.Y26.31.0005]; Tomsk State University Academic D. I. Mendeleev Fund Program [8.1.18.2015]; LiLi-NFM; Swedish Government Strategic Research Area Grant in Materials Science

Available from: 2016-06-13 Created: 2016-06-13 Last updated: 2024-01-08
Ektarawong, A., Simak, S., Hultman, L., Birch, J., Tasnádi, F., Wang, F. & Alling, B. (2016). Effects of configurational disorder on the elastic properties of icosahedral boron-rich alloys based on B6O, B13C2, and B4C, and their mixing thermodynamics. Journal of Chemical Physics, 144(13), Article ID 134503.
Open this publication in new window or tab >>Effects of configurational disorder on the elastic properties of icosahedral boron-rich alloys based on B6O, B13C2, and B4C, and their mixing thermodynamics
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2016 (English)In: Journal of Chemical Physics, ISSN 0021-9606, E-ISSN 1089-7690, Vol. 144, no 13, article id 134503Article in journal (Refereed) Published
Abstract [en]

The elastic properties of alloys between boron suboxide (B6O) and boron carbide (B13C2), denoted by (B6O)1−x(B13C2)x, as well as boron carbide with variable carbon content, ranging from B13C2 to B4C are calculated from first-principles. Furthermore, the mixing thermodynamics of (B6O)1−x(B13C2)x is studied. A superatom-special quasirandom structure approach is used for modeling different atomic configurations, in which effects of configurational disorder between the carbide and suboxide structural units, as well as between boron and carbon atoms within the units, are taken into account. Elastic properties calculations demonstrate that configurational  disorder in B13C2, where a part of the C atoms in the CBC chains substitute for B atoms in the B12 icosahedra, drastically increase the Young’s and shear modulus, as compared to an atomically ordered state, B12(CBC). These calculated elastic moduli of the disordered state are in excellent agreement with experiments. Configurational disorder between boron and carbon can also explain the experimentally observed almost constant elastic moduli of boron carbide as the carbon content is changed from B4C to B13C2. The elastic moduli of the (B6O)1−x(B13C2)x system are also practically unchanged with composition if boron-carbon disorder is taken into account. By investigating the mixing thermodynamics of the alloys, in which the Gibbs free energy is determined within the mean-field approximation for the configurational entropy, we outline the pseudo-binary phase diagram of (B6O)1−x(B13C2)x. The phase diagram reveals the existence of a miscibility gap at all temperatures up to the melting point. Also, the coexistence of B6O-rich as well as ordered or disordered B13C2-rich domains in the material prepared through equilibrium routes is predicted.

Place, publisher, year, edition, pages
American Institute of Physics (AIP), 2016
National Category
Physical Sciences
Identifiers
urn:nbn:se:liu:diva-122425 (URN)10.1063/1.4944982 (DOI)000374527900023 ()27059576 (PubMedID)
Note

Funding agencies:Swedish Research Council (VR) [621-2011-4417, 330-2014-6336, 2011-42-59]; CeNano at Linkoping University; Ministry of Education and Science of the Russian Federation in the framework of Increase Competitiveness Program of NUST "MISiS" [K3-2014-049]; LiLi-

At the time for thesis presentation publication was in status: Manuscript

Available from: 2015-11-02 Created: 2015-11-02 Last updated: 2021-12-29Bibliographically approved
Organisations
Identifiers
ORCID iD: ORCID iD iconorcid.org/0000-0002-1320-389X

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