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Organic semiconductor perylenetetracarboxylic diimide (PTCDI) electrodes for electrocatalytic reduction of oxygen to hydrogen peroxide
Linköping University, Department of Science and Technology, Physics and Electronics. Linköping University, Faculty of Science & Engineering.
Linköping University, Department of Science and Technology, Physics and Electronics. Linköping University, Faculty of Science & Engineering.
Linköping University, Department of Science and Technology, Physics and Electronics. Linköping University, Faculty of Science & Engineering.
Linköping University, Department of Science and Technology, Physics and Electronics. Linköping University, Faculty of Science & Engineering. Rudjer Boskovic Inst, Croatia.
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2018 (English)In: Chemical Communications, ISSN 1359-7345, E-ISSN 1364-548X, Vol. 54, no 16, p. 1960-1963Article in journal (Refereed) Published
Abstract [en]

Hydrogen peroxide is one of the most important industrial chemicals and there is great demand for the production of H2O2 usingmore sustainable and environmentally benign methods. We show electrochemical production of H2O2 by the reduction of O-2, enabled by an organic semiconductor catalyst, N,N-dimethyl perylenetetracarboxylic diimide (PTCDI). We make PTCDI cathodes that are capable of stable and reusable operation in aqueous electrolytes in a pH range of 1-13 with a catalytic figure of merit as high as 26 kg H2O2 per g catalyst per h. These performance and stability open new avenues for organic small molecule semiconductors as electrocatalysts.

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ROYAL SOC CHEMISTRY , 2018. Vol. 54, no 16, p. 1960-1963
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URN: urn:nbn:se:liu:diva-145755DOI: 10.1039/c7cc08471dISI: 000425531500005PubMedID: 29323369OAI: oai:DiVA.org:liu-145755DiVA, id: diva2:1192510
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Funding Agencies|Wallenberg Center for Molecular Medicine at Linkoping University

Available from: 2018-03-22 Created: 2018-03-22 Last updated: 2018-10-05

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