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Phase Transitions in Confinements: Controlling Solid to Fluid Transitions of Xenon Atoms in an On-Surface Network
Univ Basel, Switzerland.
Univ Basel, Switzerland.
Univ Basel, Switzerland.
Univ Basel, Switzerland.
Vise andre og tillknytning
2019 (engelsk)Inngår i: Small, ISSN 1613-6810, E-ISSN 1613-6829, Vol. 15, nr 3, artikkel-id 1803169Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

This study reports on "phase" transitions of Xe condensates in on-surface confinements induced by temperature changes and local probe excitation. The pores of a metal-organic network occupied with 1 up to 9 Xe atoms are investigated in their propensity to undergo "condensed solid" to "confined fluid" transitions. Different transition temperatures are identified, which depend on the number of Xe atoms in the condensate and relate to the stability of the Xe clustering in the condensed "phase." This work reveals the feature-rich behavior of transitions of confined planar condensates, which provide a showcase toward future "phase-transition" storage media patterned by self-assembly. This work is also of fundamental interest as it paves the way to real space investigations of reversible solid to fluid transitions of magic cluster condensates in an array of extremely well-defined quantum confinements.

sted, utgiver, år, opplag, sider
WILEY-V C H VERLAG GMBH , 2019. Vol. 15, nr 3, artikkel-id 1803169
Emneord [en]
phase transition of discrete number of atoms; scanning tunneling microscopy (STM); small system thermodynamics; tip-induced local excitation
HSV kategori
Identifikatorer
URN: urn:nbn:se:liu:diva-154325DOI: 10.1002/smll.201803169ISI: 000456199000017PubMedID: 30556276OAI: oai:DiVA.org:liu-154325DiVA, id: diva2:1285530
Merknad

Funding Agencies|Physics Department of the University of Basel; Swiss Nanoscience Institute; Swiss National Science Foundation [200020_162512, 206021_144991, 206021_121461, 200020_175800, 206021_113149]; Swiss Commission for Technology and Innovation (CTI) [16465.1 PFNM-NM]; Swiss Government Excellence Scholarship Program for Foreign Scholars [2013.0492]; University of Heidelberg

Tilgjengelig fra: 2019-02-04 Laget: 2019-02-04 Sist oppdatert: 2019-02-04

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