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Simulations of the thermodynamics and kinetics of NH3 at the RuO2 (110) surface
Linköping University, Department of Physics, Chemistry and Biology, Chemistry. Linköping University, Faculty of Science & Engineering.ORCID iD: 0000-0001-9455-9558
Linköping University, Department of Physics, Chemistry and Biology, Applied Sensor Science. Linköping University, Faculty of Science & Engineering.
Linköping University, Department of Physics, Chemistry and Biology, Applied Sensor Science. Linköping University, Faculty of Science & Engineering.ORCID iD: 0000-0002-2817-3574
Linköping University, Department of Physics, Chemistry and Biology, Chemistry. Linköping University, Faculty of Science & Engineering.ORCID iD: 0000-0002-5341-2637
2017 (English)In: Surface Science, ISSN 0039-6028, E-ISSN 1879-2758, Vol. 656, 9 p.77-85 p.Article in journal (Refereed) Published
Abstract [en]

•The dehydrogenation of NHless thansubscriptgreater than3less than/subscriptgreater than via a bridging O on RuOless thansubscriptgreater than2less than/subscriptgreater than(110) is rate-determining.•We can confirm the experimental results that water vapour is formed in the sensor.•OH-species are formed on the RuOless thansubscriptgreater than2less than/subscriptgreater than surface which is required for the sensor response.•A multiscale scheme is devised which can be used in a variety of applications.

Place, publisher, year, edition, pages
Elsevier, 2017. Vol. 656, 9 p.77-85 p.
Keyword [en]
Catalysis; Kinetics; Ruthenium dioxide; Sensor; Surface; Thermodynamics
National Category
Analytical Chemistry
Identifiers
URN: urn:nbn:se:liu:diva-133425DOI: 10.1016/j.susc.2016.10.006OAI: oai:DiVA.org:liu-133425DiVA: diva2:1060245
Available from: 2016-12-28 Created: 2016-12-28 Last updated: 2017-01-30

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The full text will be freely available from 2018-10-20 10:21
Available from 2018-10-20 10:21

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Erdtman, EdvinAndersson, MikeLloyd Spetz, AnitaOjamäe, Lars
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