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Naphthalenediimide Polymers with Finely Tuned In-Chain pi-Conjugation: Electronic Structure, Film Microstructure, and Charge Transport Properties
Leibniz Institute Polymerforschung Dresden eV, Germany; Technical University of Dresden, Germany; Polyera Corp, IL 60077 USA.
Linköping University, Department of Science and Technology, Physics and Electronics. Linköping University, Faculty of Science & Engineering. Polyera Corp, IL 60077 USA.ORCID iD: 0000-0001-7016-6514
University of Valencia, Spain; Ciudad University of Cantoblanco, Spain.
Stanford University, CA 94305 USA.
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2016 (English)In: ADVANCED MATERIALS, ISSN 0935-9648, Vol. 28, no 41, p. 9169-+Article in journal (Refereed) Published
Abstract [en]

Naphthalenediimide-based random copolymers (PNDI-TVTx) with different p-conjugated dithienylvinylene (TVT) versus p-nonconjugated dithienylethane (TET) unit ratios (x = 100 -amp;gt; 0%) are investigated. The PNDI-TVTx-transistor electron/hole mobilities are affected differently, a result rationalized by molecular orbital topologies and energies, with hole mobility vanishing but electron mobility decreasing only by approximate to 2.5 times when going from x = 100% to 40%.
Place, publisher, year, edition, pages
WILEY-V C H VERLAG GMBH , 2016. Vol. 28, no 41, p. 9169-+
National Category
Condensed Matter Physics
Identifiers
URN: urn:nbn:se:liu:diva-134311DOI: 10.1002/adma.201602923ISI: 000391174400012PubMedID: 27572671OAI: oai:DiVA.org:liu-134311DiVA, id: diva2:1071680
Note

Funding Agencies|DFG within CoE cfaed; Advanced Functional Materials Center at Linkoping University [2009-00971]; VINNOVA [2015-04859]; MINECO [CTQ2014-58801]; CEI UAM+CSIC; DOE [DE-AC02-05CH11231]; Paul and Daisy Soros Fellowship for New Americans; NSF-GFRP; NSF (CBET) [1510481]

Available from: 2017-02-06 Created: 2017-02-03 Last updated: 2017-02-14Bibliographically approved

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