Phonon and electron contributions to the thermal conductivity of VNx epitaxial layersShow others and affiliations
2017 (English)In: Physical Review Materials, E-ISSN 2475-9953, Vol. 1, no 6, article id 065002Article in journal (Refereed) Published
Abstract [en]
Thermal conductivities of VNx/MgO(001) (0.76 amp;lt;= x amp;lt;= 1.00) epitaxial layers, grown by reactive magnetron sputter deposition, are measured in the temperature range 300 amp;lt; T amp;lt; 1000 K using time-domain thermore-flectance (TDTR). Data for the total thermal conductivity are compared to the electronic contribution to the thermal conductivity calculated from the measured electrical conductivity, the Wiedemann-Franz law, and an estimate of the temperature dependence of the Lorenz number L(T). The total thermal conductivity is dominated by electron contribution and varies between 13 W m(-1) K-1 at x = 0.76 and 20 W m(-1) K-1 at x = 1.00 for T = 300 K and between 25 and 35 W m(-1) K-1 for T = 1000 K. The lattice thermal conductivity vs x ranges from 5 to 7 W m(-1) K-1 at 300 K and decreases by 20% at 500 K. The low magnitude and weak temperature dependence of the lattice thermal conductivity are attributed to strong electron-phonon coupling in VN.
Place, publisher, year, edition, pages
AMER PHYSICAL SOC , 2017. Vol. 1, no 6, article id 065002
National Category
Condensed Matter Physics
Identifiers
URN: urn:nbn:se:liu:diva-143732DOI: 10.1103/PhysRevMaterials.1.065002ISI: 000416597100002OAI: oai:DiVA.org:liu-143732DiVA, id: diva2:1166718
Note
Funding Agencies|Swedish Research Council (VR) [2009-00971, 2013-4018, 2014-5790]; Swedish Government Strategic Research Area Grant in Materials Science (SFO Mat-LiU) on Advanced Functional Materials; Olle Engkvist Foundation
2017-12-152017-12-152021-12-28