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The influence of ortho-methyl substitution in organometallic self-assembly - a comparative study on Cu(111) vs. Ag(111)
Deutsch Museum, Germany; Tech Univ Munich, Germany.
Bavarian Acad Sci and Humanities, Germany.
Linköping University, Department of Physics, Chemistry and Biology, Theoretical Physics. Linköping University, Faculty of Science & Engineering.ORCID iD: 0000-0002-1345-0006
Univ Siegen, Germany.
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2018 (English)In: Chemical Communications, ISSN 1359-7345, E-ISSN 1364-548X, Vol. 54, no 70, p. 9745-9748Article in journal (Refereed) Published
Abstract [en]

Metal surface-induced dehalogenation of precursors is known to initiate self-assembly of organometallic networks, where tectons are connected via carbon-metal-carbon (C-M-C) bonds. Even though reversibility of the C-M-C bonds facilitates structural equilibration, defects associated with highly bent organometallic linkages are still commonly observed. By introducing a steric hindrance to reduce the C-M-C bond angle flexibility, we find well ordered organometallic networks of an ortho-methyl substituted 1,3,5-tris(p-bromophenyl)-benzene analogue on Cu(111) after room-temperature (RT) deposition and on Ag(111) after annealing.

Place, publisher, year, edition, pages
ROYAL SOC CHEMISTRY , 2018. Vol. 54, no 70, p. 9745-9748
National Category
Inorganic Chemistry
Identifiers
URN: urn:nbn:se:liu:diva-151185DOI: 10.1039/c8cc04854aISI: 000442872000007PubMedID: 30109325OAI: oai:DiVA.org:liu-151185DiVA, id: diva2:1248626
Available from: 2018-09-17 Created: 2018-09-17 Last updated: 2018-09-17

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