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Reproducible Planar Heterojunction Solar Cells Based on One-Step Solution-Processed Methylammonium Lead Halide Perovskites
Linköping University, Department of Physics, Chemistry and Biology, Biomolecular and Organic Electronics. Linköping University, Faculty of Science & Engineering. Univ Oxford, England.
Univ Oxford, England.
Univ Oxford, England; Univ Lincoln, England.
Univ Oxford, England.
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2017 (English)In: Chemistry of Materials, ISSN 0897-4756, E-ISSN 1520-5002, Vol. 29, no 1, p. 462-473Article in journal (Refereed) Published
Abstract [en]

Metal halide perovskites have been demonstrated as one of the most promising materials for low-cost and high-performance photovoltaic applications. However, due to the susceptible crystallization process of perovskite films on planar substrates and the high sensitivity of the physical and optoelectronic nature of the internal interfaces within the devices, researchers in different laboratories still experience poor reproducibility in fabricating efficient perovskite solar cells with planar heterojunction device structures. In this method paper, we present detailed information on the reagents, equipment, and procedures for the fabrication of planar perovskite solar cells in both "regular" n-i-p and "inverted" p-i-n architectures based on one-step solution-processed methylammonium lead triiodide (MAPbI(3)) perovskite films. We discuss key parameters affecting the crystallization of perovskite and the device interfaces. This method paper will provide a guideline for the reproducible fabrication of planar heterojunction solar cells based on MAPbI3 perovskite films. We believe that the shared experience on MA-based perovskite films and planar solar cells will be also useful for the optimization process of perovskites with varied compositions, and other emerging perovskite-based optoelectronic devices.

Place, publisher, year, edition, pages
AMER CHEMICAL SOC , 2017. Vol. 29, no 1, p. 462-473
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Other Materials Engineering
Identifiers
URN: urn:nbn:se:liu:diva-153804DOI: 10.1021/acs.chemmater.6b05159ISI: 000391898300034OAI: oai:DiVA.org:liu-153804DiVA, id: diva2:1277879
Note

Funding Agencies|UK engineering and Physical Sciences Research Council (EPSRC) [EP/P02484X/1, EP/M024881/1, EP/M015254/1, EP/M014797/1, EP/M005143/1, EP/M023532/1, EP/L024667/1]; Supergen Super Solar project; Carl Tryggers Stiftelse; VINNMER Fellow; Marie Sklodowska-Curie Fellow

Available from: 2019-01-11 Created: 2019-01-11 Last updated: 2019-03-06

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