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Atomically Layered and Ordered Rare-Earth i-MAX Phases: A New Class of Magnetic Quaternary Compounds
Linköping University, Department of Physics, Chemistry and Biology, Thin Film Physics. Linköping University, Faculty of Science & Engineering.
Linköping University, Department of Physics, Chemistry and Biology, Thin Film Physics. Linköping University, Faculty of Science & Engineering.
Linköping University, Department of Physics, Chemistry and Biology, Thin Film Physics. Linköping University, Faculty of Science & Engineering.ORCID iD: 0000-0001-5036-2833
Linköping University, Department of Physics, Chemistry and Biology, Thin Film Physics. Linköping University, Faculty of Science & Engineering. Oak Ridge Natl Lab, TN 37831 USA.
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2019 (English)In: Chemistry of Materials, ISSN 0897-4756, E-ISSN 1520-5002, Vol. 31, no 7, p. 2476-2485Article in journal (Refereed) Published
Abstract [en]

In 2017, we discovered quaternary i-MAX phases atomically layered solids, where M is an early transition metal, A is an A group element, and X is C-with a ((M2/3M1/32)-M-1)(2)AC chemistry, where the M-1 and M-2 atoms are in-plane ordered. Herein, we report the discovery of a class of magnetic i-MAX phases in which bilayers of a quasi-2D magnetic frustrated triangular lattice overlay a Mo honeycomb arrangement and an Al Kagome lattice. The chemistry of this family is (Mo2/3RE1/3)(2)AlC, and the rare-earth, RE, elements are Ce, Pr, Nd, Sm, Gd, Tb, Dy, Ho, Er, Tm, and Lu. The magnetic properties were characterized and found to display a plethora of ground states, resulting from an interplay of competing magnetic interactions in the presence of magnetocrystalline anisotropy.

Place, publisher, year, edition, pages
AMER CHEMICAL SOC , 2019. Vol. 31, no 7, p. 2476-2485
National Category
Condensed Matter Physics
Identifiers
URN: urn:nbn:se:liu:diva-157225DOI: 10.1021/acs.chemmater.8b05298ISI: 000464477100029OAI: oai:DiVA.org:liu-157225DiVA, id: diva2:1324349
Note

Funding Agencies|Knut and Alice Wallenberg (KAW) Foundation [KAW 2015.0043]; Swedish Research Council [642-2013-8020, 2015-00607, 621-2014-4890]; Swedish Government Strategic Research Area in Materials Science on Functional Materials at Linkoping University (Faculty Grant SFO-Mat-LiU) [2009-00971]; DFG [SA 3095/2-1]; IAEC Pazy Foundation Grant; NSF [DMR-1740795]

Available from: 2019-06-13 Created: 2019-06-13 Last updated: 2019-06-13

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Tao, QuanzhengLu, JunDahlqvist, MartinMockuté, AurelijaPetruhins, AndrejsMeshkian, RaheleHultman, LarsBarsoum, MichelRosén, Johanna
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