We continue our investigation on general large deviation principles (LDPs) for longest runs. Previously, a general LDP for the longest success run in a sequence of independent Bernoulli trails was derived in [Z. Liu and X. Yang, A general large deviation principle for longest runs, Statist. Probab. Lett. 110 (2016), 128-132]. In the present note, we establish a general LDP for the longest success run in a two-state (success or failure) Markov chain which recovers the previous result in the aforementioned paper. The main new ingredient is to implement suitable estimates of the distribution function of the longest success run recently established in [Z. Liu and X. Yang, On the longest runs in Markov chains, Probab. Math. Statist. 38 (2018), no. 2, 407-428].