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Resonance enhanced Raman scattering from the complex electric-dipole polarizability: A theoretical study on N-2
Royal Institute of Technology.
Royal Institute of Technology.
Linköping University, Department of Physics, Chemistry and Biology, Computational Physics . Linköping University, The Institute of Technology.
2009 (English)In: CHEMICAL PHYSICS LETTERS, ISSN 0009-2614 , Vol. 468, no 4-6, 119-123 p.Article in journal (Refereed) Published
Abstract [en]

An expression for resonant molecular Raman scattering in terms of the complex electric-dipole polarizability tensor is presented and implemented with first principles complex polarization propagator theory. The theory reveals the strong role of phase delays of the detected Raman radiation in the resonant case. Application on gaseous nitrogen predicts a Raman scattering enhancement of circa 104 in the resonance regions of the b(1)Pi(u) and b (1)Sigma(+)(u) states as compared to the nonresonant case.

Place, publisher, year, edition, pages
2009. Vol. 468, no 4-6, 119-123 p.
National Category
Natural Sciences
URN: urn:nbn:se:liu:diva-16521DOI: 10.1016/j.cplett.2008.11.063OAI: diva2:158129
Available from: 2009-01-30 Created: 2009-01-30 Last updated: 2009-01-30

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Norman , Patrick
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