liu.seSearch for publications in DiVA
Change search
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • oxford
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf
Spectroscopic studies of InGaAs/GaAs/A1GaAs quantum dots and wires
Linköping University, Department of Physics, Measurement Technology, Biology and Chemistry. Linköping University, The Institute of Technology.
2004 (English)Doctoral thesis, comprehensive summary (Other academic)
Abstract [en]

It is demonstrated that the photoluminescence (PL) spectra of single selfassembled lnAs/GaAs quantum dots (QDs) are very sensitive to excitation energy and crystal temperature, which is explained in terms of modulation of the effective diffusivity of the photogenerated carriers affecting the capture probability into theQD. This effect results in a population of the QD with excess electrons, and can be used as a simple tool to create and study charged exciton complexes. Charged excitons of the studied QDs are thus identified and found to be in agreement with a theoretical model.

An alternative way of optically charging single QDs with extra electrons at low temperatures is also presented, relying on the presence of residual acceptor-atoms in the barrier in the vicinity of the dot. The acceptors define a distinct threshold transition energy below the barrier band gap. This threshold energy is dependent on the binding energies of the acceptors, i.e. which common acceptors in GaAs are present in the vicinity of the studied QD. Exciting with a photon energy above (below) this threshold creates negative (neutral) excitons in the QD, and is a very efficient tool to study charged exciton complexes.

It has been proposed that the properties of excitons in low-dimensional quantum structures such as quantum wires (QWRs) can be described by a fractional dimension with a value depending on the confinement. This theory has been applied to V-groove GaAs /A1GaAs QWRs in order to obtain the absorption spectrum, and the achieved result is verified by comparison with a more complete model as well as with PL excitation (PLE) experiments. It is found that the fractional dimension theory offers an efficient and accurate way to determine the absorption spectrum, although situations of strong intersubband couplings are identified where the theory naturally fails, at least to some extent.

Asymmetric double V-groove GaAs/A1GaAs quantum wires light-emitting diode (LED) systems have been subjected to electroluminescence (EL) and PLE measurements, revealing a very efficient charge and exciton transfer from the narrow tothe wide QWR at low temperatures, despite a 7 nm thick tunneling barrier. The tunneling efficiency is found to be comparable for both electrons and holes, and evidence for tunneling is revealed up to room temperature. Furthermore, PL and PLE studies on analogous QWR systems with various thicknesses of the barriers demonstrate, when compared with a numerical calculation of the tunneling efficiency, that the carrier transfer between the QWRs can be explained by conventional tunneling. The effect of exciton leakage often present between the quantum wells is thus not present here.

Finally GaAs/A1GaAs and InGaAs/GaAs/A1GaAs V-groove quantum wire LEDs are subjected to magnetic fields for different configurations of the field with respect to the wire axis. The ground state diamagnetic shifts are determined by ELand compared with the results of a proposed two-band exciton model. It is found that this model cannot in a satisfactory way explain the experimental data, since it predicts too large shifts (about a factor of two for the GaAs/A1GaAs QWRs). One possible reason for this is the neglected valence band mixing in the exciton approach, which issupported by a better agreement for the InGaAs/GaAs/A1GaAs QWRs where the strain splits the valence bands and weakens the effects of valence band mixing.

Place, publisher, year, edition, pages
Linköping: Linköping University , 2004. , p. 52
Series
Linköping Studies in Science and Technology. Dissertations, ISSN 0345-7524 ; 892
National Category
Theoretical Chemistry
Identifiers
URN: urn:nbn:se:liu:diva-179262Libris ID: 9614544ISBN: 9185295264 (print)OAI: oai:DiVA.org:liu-179262DiVA, id: diva2:1594378
Public defence
2004-09-24, hörsal Planck, Fysikhuset, Linköpings universitet, Linköping, 10:15
Opponent
Note

All or some of the partial works included in the dissertation are not registered in DIVA and therefore not linked in this post.

Available from: 2021-09-29 Created: 2021-09-15 Last updated: 2023-02-24Bibliographically approved
List of papers
1. Fractional-dimensional excitonic absorption theory applied to real V-groove quantum wires
Open this publication in new window or tab >>Fractional-dimensional excitonic absorption theory applied to real V-groove quantum wires
2004 (English)In: 27th International Conference on the Physics of Semiconductors ICPS-27,2004, 2004Conference paper, Published paper (Other academic)
National Category
Natural Sciences
Identifiers
urn:nbn:se:liu:diva-44060 (URN)75496 (Local ID)75496 (Archive number)75496 (OAI)
Available from: 2009-10-10 Created: 2009-10-10 Last updated: 2021-09-15
2. Electroluminescence and photoluminescence excitation study of asymmetric coupled GaAs/AlxGa1-xAs V-groove quantum wires
Open this publication in new window or tab >>Electroluminescence and photoluminescence excitation study of asymmetric coupled GaAs/AlxGa1-xAs V-groove quantum wires
Show others...
2004 (English)In: Physical Review B. Condensed Matter and Materials Physics, ISSN 1098-0121, E-ISSN 1550-235X, Vol. 70, no 4Article in journal (Refereed) Published
Abstract [en]

We have studied systems of asymmetric coupled GaAs V-groove quantum wires p-i-n diodes, in which the electrons and holes are injected into different wires. Despite the use of a 7 nm thick AlGaAs tunnel barrier, and although we demonstrate that holes tunnel more slowly than electrons, we observe a very efficient and fast tunneling between the quantum wires (QWR's). We attribute this to the achievement of a resonance between hole levels in the two QWR's. Photoluminescence excitation experiments are compared with accurate calculations of the excitonic absorption yielding a level of carrier transfer of nearly 100%. Temperature-dependent electroluminescence exhibits clear effects of tunneling up to room temperature but cannot distinguish separate electron/hole tunneling from exciton tunneling.

National Category
Natural Sciences
Identifiers
urn:nbn:se:liu:diva-44028 (URN)10.1103/PhysRevB.70.045302 (DOI)75462 (Local ID)75462 (Archive number)75462 (OAI)
Available from: 2009-10-10 Created: 2009-10-10 Last updated: 2021-09-15

Open Access in DiVA

No full text in DiVA

Search in DiVA

By author/editor
Karlsson, Fredrik
By organisation
Department of Physics, Measurement Technology, Biology and ChemistryThe Institute of Technology
Theoretical Chemistry

Search outside of DiVA

GoogleGoogle Scholar

isbn
urn-nbn

Altmetric score

isbn
urn-nbn
Total: 62 hits
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • oxford
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf