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Orbital-specific dynamic charge transfer from Fe(II)-tetraphenylporphyrin molecules to molybdenum disulfide substrates
Linköping University, Department of Physics, Chemistry and Biology. Linköping University, The Institute of Technology.
Linköping University, Department of Physics, Chemistry and Biology. Linköping University, The Institute of Technology.
Department of Synchrotron Radiation Research, Institute of Physics, University of Lund, Lund, Sweden.
Department of Physics, Uppsala University, Uppsala, Sweden.
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2005 (English)In: Physical Review B. Condensed Matter and Materials Physics, ISSN 1098-0121, E-ISSN 1550-235X, Vol. 72, no 3, 35448- p.Article in journal (Refereed) Published
Abstract [en]

Orbital-specific femtosecond charge transfer dynamics between Fe(II)-tetraphenylporphyrin molecules and semimetallic molybdenum disulfide substrates is investigated using core-level resonant photoemission spectroscopy. The electronic coupling to the substrate and the efficiency of charge transport across the interface is found to be different for the individual molecular electronic subsystems. In particular, electrons excited at the phenyl substituents are transferred within 3–6 fs, while hopping from the porphyrin ring is slower than 30 fs.

Place, publisher, year, edition, pages
2005. Vol. 72, no 3, 35448- p.
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Natural Sciences
Identifiers
URN: urn:nbn:se:liu:diva-30230DOI: 10.1103/PhysRevB.72.035448Local ID: 15734OAI: oai:DiVA.org:liu-30230DiVA: diva2:251052
Available from: 2009-10-09 Created: 2009-10-09 Last updated: 2017-12-13

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de Jong, Michel PFriedlein, RainerOsikowicz, WojciechTengstedt, CarlJönsson, StinaFahlman, MatsSalaneck, William R

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de Jong, Michel PFriedlein, RainerOsikowicz, WojciechTengstedt, CarlJönsson, StinaFahlman, MatsSalaneck, William R
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Department of Physics, Chemistry and BiologyThe Institute of TechnologyDepartment of Science and Technology
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Physical Review B. Condensed Matter and Materials Physics
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