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Growth of fullerene-like carbon nitride thin solid films consisting of cross-linked nano-onions
Linköping University, The Institute of Technology. Linköping University, Department of Physics, Chemistry and Biology, Thin Film Physics.
Linköping University, The Institute of Technology. Linköping University, Department of Physics, Chemistry and Biology, Thin Film Physics.ORCID iD: 0000-0002-2837-3656
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2001 (English)In: Applied Physics Letters, ISSN 0003-6951, E-ISSN 1077-3118, Vol. 79, no 16, 2639-2641 p.Article in journal (Refereed) Published
Abstract [en]

Fullerene-like CNx (x˜0.12) thin solid films were deposited by reactive magnetron sputtering of graphite in a nitrogen and argon discharge on cleaved NaCl and Si(001) substrates at 450°C. As-deposited films consist of 5 nm diam CNx nano-onions with shell sizes corresponding to Goldberg polyhedra determined by high-resolution transmission electron microscopy. Electron energy loss spectroscopy revealed that N incorporation is higher in the core of the onions than at the perimeter. N incorporation promotes pentagon formation and provides reactive sites for interlinks between shells of the onions. A model is proposed for the formation of CNx nano-onions by continuous surface nucleation and growth of hemispherical shells. © 2001 American Institute of Physics.

Place, publisher, year, edition, pages
2001. Vol. 79, no 16, 2639-2641 p.
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Engineering and Technology
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URN: urn:nbn:se:liu:diva-47242DOI: 10.1063/1.1412596OAI: oai:DiVA.org:liu-47242DiVA: diva2:268138
Available from: 2009-10-11 Created: 2009-10-11 Last updated: 2017-12-13

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Neidhardt, JörgHultman, Lars

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