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Direct ESR detection of S=3/2 states for nitrosyl iron complexes in FeZSM-5 zeolites
Boreskov Institute of Catalysis, Novosibirsk 630090, Russian Federation.
Boreskov Institute of Catalysis, Novosibirsk 630090, Russian Federation.
Linköping University, The Institute of Technology. Linköping University, Department of Physics, Chemistry and Biology, Chemical Physics .
2001 (English)In: Chemical Physics Letters, ISSN 0009-2614, E-ISSN 1873-4448, Vol. 333, no 1-2, 41-44 p.Article in journal (Refereed) Published
Abstract [en]

The formation of paramagnetic complexes between Fe2+ ions and NO molecules with total spin S=3/2 has been observed in FeZSM-5 zeolites. These complexes exhibit a typical ESR signal with a component at g=4.0 and are spectroscopically similar to those observed in iron-containing enzymes. Such spin states of Fe ions have not been reported for heterogeneous catalysts. The application of NO as a spin probe for investigation of the state of low-valence Fe ions in zeolite matrices is discussed. © 2001 Elsevier Science B.V.

Place, publisher, year, edition, pages
2001. Vol. 333, no 1-2, 41-44 p.
National Category
Engineering and Technology
Identifiers
URN: urn:nbn:se:liu:diva-47485DOI: 10.1016/S0009-2614(00)01357-9OAI: oai:DiVA.org:liu-47485DiVA: diva2:268381
Available from: 2009-10-11 Created: 2009-10-11 Last updated: 2017-12-13

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Lund, Anders

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