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Iron-polyaniline interfaces: Implications for corrosion protection
Linköping University, The Institute of Technology. Linköping University, Department of Physics, Chemistry and Biology, Surface Physics and Chemistry .
Linköping University, The Institute of Technology. Linköping University, Department of Science and Technology.ORCID iD: 0000-0001-8845-6296
Linkoping Univ, Dept Sci & Technol, SE-60174 Norrkoping, Sweden Linkoping Univ, Dept Phys, SE-58183 Linkoping, Sweden Ohio State Univ, Dept Phys, Columbus, OH 43210 USA Univ Mons, Serv Chim Mat Nouveaux, B-7000 Mons, Belgium Drexel Univ, Dept Chem, Philadelphia, PA 19104 USA.
Linkoping Univ, Dept Sci & Technol, SE-60174 Norrkoping, Sweden Linkoping Univ, Dept Phys, SE-58183 Linkoping, Sweden Ohio State Univ, Dept Phys, Columbus, OH 43210 USA Univ Mons, Serv Chim Mat Nouveaux, B-7000 Mons, Belgium Drexel Univ, Dept Chem, Philadelphia, PA 19104 USA.
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2003 (English)In: American Chemical Society Symposium Series (ACS), ISSN 0097-6156, E-ISSN 1947-5918, Vol. 843, 76-89 p.Article in journal (Refereed) Published
Abstract [en]

The early stages of interface formation between iron and a three-ring model molecule (trimer) of emeraldine base form of polyaniline (EB) were investigated using theoretical (DFT) and experimental (XPS) methods: Iron atoms were sputter-deposited in ultra high vacuum onto thin oligomer films, with X-ray photoelectron spectroscopy (XPS) core level spectra taken after each deposition. Similar studies were carried out for Fe sputter-deposited on EB polymer films as well. Based on the chemical shifts of the core level peaks and the theoretical results, iron was determined to donate charge (e(-)) into the trimer and EB films. The reverse case where thin films of trimer and EB were deposited on iron also was studied. The C(1s) core level shake up spectra show that the pi-electronic structure is modified for trimer and EB coatings on iron as compared to coatings on gold. (C) 2003 American Chemical Society.

Place, publisher, year, edition, pages
2003. Vol. 843, 76-89 p.
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Engineering and Technology
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URN: urn:nbn:se:liu:diva-48668OAI: oai:DiVA.org:liu-48668DiVA: diva2:269564
Available from: 2009-10-11 Created: 2009-10-11 Last updated: 2017-12-12

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Fahlman, MatsCrispin, Xavier

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