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EPR of trans-stilbene radical cations formed in zeolite cavities: a new approach to study the zeolite void space
Univ Venice, Dipartimento Chim, I-30123 Venice, Italy Univ Padua, Dipartimento Chim Fis, I-35131 Padua, Italy Linkoping Univ, Dept Chem Phys, S-58183 Linkoping, Sweden Hiroshima Univ, Dept Appl Chem, Fac Engn, Higashihiroshima 7398527, Japan Univ Modena, Dipartimento Chim, I-41100 Modena, Italy.
Univ Venice, Dipartimento Chim, I-30123 Venice, Italy Univ Padua, Dipartimento Chim Fis, I-35131 Padua, Italy Linkoping Univ, Dept Chem Phys, S-58183 Linkoping, Sweden Hiroshima Univ, Dept Appl Chem, Fac Engn, Higashihiroshima 7398527, Japan Univ Modena, Dipartimento Chim, I-41100 Modena, Italy.
Univ Venice, Dipartimento Chim, I-30123 Venice, Italy Univ Padua, Dipartimento Chim Fis, I-35131 Padua, Italy Linkoping Univ, Dept Chem Phys, S-58183 Linkoping, Sweden Hiroshima Univ, Dept Appl Chem, Fac Engn, Higashihiroshima 7398527, Japan Univ Modena, Dipartimento Chim, I-41100 Modena, Italy.
Univ Venice, Dipartimento Chim, I-30123 Venice, Italy Univ Padua, Dipartimento Chim Fis, I-35131 Padua, Italy Linkoping Univ, Dept Chem Phys, S-58183 Linkoping, Sweden Hiroshima Univ, Dept Appl Chem, Fac Engn, Higashihiroshima 7398527, Japan Univ Modena, Dipartimento Chim, I-41100 Modena, Italy.
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2000 (English)In: Physical Chemistry, Chemical Physics - PCCP, ISSN 1463-9076, E-ISSN 1463-9084, Vol. 2, no 20, 4823-4828 p.Article in journal (Refereed) Published
Abstract [en]

trans-Stilbene was adsorbed in the cavities of H-ZSM-5, H-MOR and H-BEA zeolites, originating monomeric and dimeric radical cations that were studied by EPR spectroscopy. The H-BEA samples were pretreated at three progressively higher temperatures. Simulation of the spectra allowed the evaluation of the relative amounts of monomers and dimers. The nature, quantity and relative amount of monomeric and dimeric radical species were correlated to chemical and dimensional modifications of zeolite channels caused by the dealumination of the zeolite structure and extra-framework aluminium species formation.

Place, publisher, year, edition, pages
2000. Vol. 2, no 20, 4823-4828 p.
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Natural Sciences
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URN: urn:nbn:se:liu:diva-49567OAI: oai:DiVA.org:liu-49567DiVA: diva2:270463
Available from: 2009-10-11 Created: 2009-10-11 Last updated: 2017-12-12

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