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X-ray magnetic circular dichroism and resonant photomission of V(TCNE)x hybrid magnets
Linköping University, The Institute of Technology. Linköping University, Department of Science and Technology.
Linköping University, The Institute of Technology. Linköping University, Department of Physics, Chemistry and Biology, Surface Physics and Chemistry .
Linköping University, The Institute of Technology. Linköping University, Department of Science and Technology.
Linköping University, The Institute of Technology. Linköping University, Department of Science and Technology.
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2006 (English)In: Physical Review Letters, ISSN 0031-9007, E-ISSN 1079-7114, Vol. 96, no 5Article in journal (Refereed) Published
Abstract [en]

Thin films of V(TCNE)x were deposited in ultrahigh vacuum using a film growth technique based on in situ chemical vapor deposition of tetracyanoethylene, TCNE, and bis-benzene vanadium, V(C6H6)2. The in situ preparation method enabled, for the first time, experimental analysis of oxygen-free films. X-ray magnetic circular dichroism measurements recorded at the V L2,3 edge confirmed room temperature magnetic ordering. A combination of conventional photoelectron spectroscopy (PES) and resonant photoemission (RPE) measured at the V L3 edge shows that the highest occupied electronic state is V(3d) derived. The rearrangements of the TCNE- related valence electronic states observed in PES and the evidence of V(3d) and TCNE- p(p*) orbital overlap contained in RPE spectra, indicate that strong, covalent type bonding occurs between the vanadium and the TCNE molecules. © 2006 The American Physical Society.

Place, publisher, year, edition, pages
2006. Vol. 96, no 5
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Engineering and Technology
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URN: urn:nbn:se:liu:diva-50299DOI: 10.1103/PhysRevLett.96.057209OAI: oai:DiVA.org:liu-50299DiVA: diva2:271195
Available from: 2009-10-11 Created: 2009-10-11 Last updated: 2017-12-12

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Tengstedt, Carlde Jong, Michel PKanciurzewska, AnnaCarlegrim, ElinFahlman, Mats

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