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Hydrogen Bond Interaction between Self-Assembled Monolayers and Adsorbed Water Molecules and Its Implications for Cluster Formation
Linköping University, Department of Physics, Chemistry and Biology, Applied Physics. Linköping University, The Institute of Technology.ORCID iD: 0000-0001-5365-6140
Linköping University, Department of Physics, Chemistry and Biology, Applied Physics. Linköping University, The Institute of Technology.
Linköping University, Department of Physics, Chemistry and Biology, Applied Physics. Linköping University, The Institute of Technology.
1995 (English)In: Journal of Physical Chemistry B, ISSN 1520-6106, E-ISSN 1520-5207, Vol. 99, no 39, 14198-14200 p.Article in journal (Refereed) Published
Abstract [en]

Infrared spectroscopy is used to investigate the adsorption of D2O onto self-assembled monolayers of methyl 16-mercaptohexadecanoate on gold. The D2O molecules are shown to interact with the carbonyl oxygens of the monolayer, forming hydrogen bonds and causing a structural rearrangement of the CO2CH3 terminal group. The number of hydrogen bonds decreases as the amorphous-like, essentially flat (two-dimensional) ice overlayer that forms at 100 K changes into polycrystalline-like ice upon annealing at 140 K. This decrease is a consequence of the formation of three-dimensional ice clusters, which leaves a large fraction of the monolayer surface bare.

Place, publisher, year, edition, pages
AMER CHEMICAL SOC , 1995. Vol. 99, no 39, 14198-14200 p.
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Engineering and Technology
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URN: urn:nbn:se:liu:diva-76342DOI: 10.1021/j100039a002ISI: A1995RX87500002OAI: oai:DiVA.org:liu-76342DiVA: diva2:513818
Available from: 2012-04-03 Created: 2012-04-03 Last updated: 2017-12-07

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Engquist, IsakLiedberg, Bo

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