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Use of two-dimensional photoelectron spectroscopy in the decomposition of an inner-shell excitation spectrum broadened by super-Coster-Kronig decay
CNR, Italy .
Linköping University, Department of Physics, Chemistry and Biology, Computational Physics. Linköping University, The Institute of Technology.
CNR, Italy .
CNR, Italy .
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2013 (English)In: Physical Review A. Atomic, Molecular, and Optical Physics, ISSN 1050-2947, E-ISSN 1094-1622, Vol. 88, no 6, 062502- p.Article in journal (Refereed) Published
Abstract [en]

The Ge 3p core excitation spectrum of the n-butylgermane molecule only reveals two peaks, whereas the rest of the fine structure is obscured due to the large lifetime broadenings of core-excited states. A two-dimensional presentation of resonant photoemission spectra allows us to observe some other resonances. The interpretation of experimental results is supported by ab initio calculations conducted at the four-component relativistic level of theory with full account made for spin-orbit interactions already in the zeroth-order Hamiltonian.

Place, publisher, year, edition, pages
American Physical Society , 2013. Vol. 88, no 6, 062502- p.
National Category
Engineering and Technology
URN: urn:nbn:se:liu:diva-103294DOI: 10.1103/PhysRevA.88.062502ISI: 000328567900007OAI: diva2:688489
Available from: 2014-01-17 Created: 2014-01-16 Last updated: 2014-01-29

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