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Hybrid Interface States and Spin Polarization at Ferromagnetic Metal-Organic Heterojunctions: Interface Engineering for Efficient Spin Injection in Organic Spintronics
Linköping University, Department of Physics, Chemistry and Biology, Surface Physics and Chemistry. Linköping University, The Institute of Technology.
Linköping University, Department of Physics, Chemistry and Biology, Surface Physics and Chemistry. Linköping University, The Institute of Technology.
CiC NanoGUNE Consolider, Spain .
CNR, Italy .
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2014 (English)In: Advanced Functional Materials, ISSN 1616-301X, E-ISSN 1616-3028, Vol. 24, no 30, 4812-4821 p.Article in journal (Refereed) Published
Abstract [en]

Ferromagnetic metal-organic semiconductor (FM-OSC) hybrid interfaces have been shown to play an important role for spin injection in organic spintronics. Here, 11,11,12,12-tetracyanonaptho-2,6-quinodimethane (TNAP) is introduced as an interfacial layer in Co-OSCs heterojunctions with an aim to tune the spin injection. The Co/TNAP interface is investigated by use of X-ray and ultraviolet photoelectron spectroscopy (XPS/UPS), near edge X-ray absorption fine structure (NEXAFS) and X-ray magnetic circular dichroism (XMCD). Hybrid interface states (HIS) are observed at Co/TNAP interfaces, resulting from chemical interactions between Co and TNAP. The energy level alignment at the Co/TNAP/OSCs interface is also obtained, and a reduction of the hole injection barrier is demonstrated. XMCD results confirm sizeable spin polarization at the Co/TNAP hybrid interface.

Place, publisher, year, edition, pages
Wiley-VCH Verlag , 2014. Vol. 24, no 30, 4812-4821 p.
National Category
Physical Sciences
Identifiers
URN: urn:nbn:se:liu:diva-110478DOI: 10.1002/adfm.201400125ISI: 000340549900011OAI: oai:DiVA.org:liu-110478DiVA: diva2:746962
Note

Funding Agencies|European Union [263104]; Swedish Research Council; Swedish Research Council (Linneus center); Knut and Alice Wallenberg Foundation

Available from: 2014-09-15 Created: 2014-09-12 Last updated: 2017-12-05

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Shi, ShengweiSun, ZhengyiLiu, XianjieFahlman, Mats

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Surface Physics and ChemistryThe Institute of Technology
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