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X-ray and Electron Spectroscopy of Water
Linköping University, Department of Physics, Chemistry and Biology, Theoretical Chemistry. Linköping University, Faculty of Science & Engineering.
University of Tokyo, Japan.
Institute Molecular Science, Japan.
University of Nottingham, England.
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2016 (English)In: Chemical Reviews, ISSN 0009-2665, E-ISSN 1520-6890, Vol. 116, no 13, 7551-7569 p.Article, review/survey (Refereed) PublishedText
Abstract [en]

Here we present an overview of recent developments of X-ray and electron spectroscopy to probe water at different temperatures. Photon-induced ionization followed by detection of electrons from either the 0 is level or the valence band is the basis of photoelectron spectroscopy. Excitation between the 0 is and the unoccupied states or occupied states is utilized in X-ray absorption and X-ray emission spectroscopies. These techniques probe the electronic structure of the liquid phase and show sensitivity to the local hydrogen-bonding structure. Both experimental aspects related to the measurements and theoretical simulations to assist in the interpretation are discussed in detail. Different model systems are presented such as the different bulk phases of ice and various adsorbed monolayer structures on metal surfaces.

Place, publisher, year, edition, pages
AMER CHEMICAL SOC , 2016. Vol. 116, no 13, 7551-7569 p.
National Category
Atom and Molecular Physics and Optics
Identifiers
URN: urn:nbn:se:liu:diva-130381DOI: 10.1021/acs.chemrev.5b00672ISI: 000379794000005PubMedID: 27244473OAI: oai:DiVA.org:liu-130381DiVA: diva2:952762
Note

Funding Agencies|Royal Swedish Academy of Sciences through Nobel Institutes for Physics and Chemistry; Swedish Research Council; Department of Physics at Stockholm University

Available from: 2016-08-15 Created: 2016-08-05 Last updated: 2016-08-15

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