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  • 1.
    Fabiano, Simone
    et al.
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Abdollahi Sani, Negar
    Linköpings universitet, Institutionen för teknik och naturvetenskap. Linköpings universitet, Tekniska fakulteten. RISE Acreo, Sweden.
    Kawahara, Jun
    RISE Acreo, Sweden; LINTEC Corp, Japan.
    Kergoat, Loig
    Linköpings universitet, Institutionen för teknik och naturvetenskap. Linköpings universitet, Tekniska fakulteten. Aix Marseille University, France.
    Nissa, Josefin
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Engquist, Isak
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Crispin, Xavier
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Berggren, Magnus
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Ferroelectric polarization induces electronic nonlinearity in ion-doped conducting polymers2017Inngår i: Science Advances, ISSN 0036-8156, E-ISSN 2375-2548, Vol. 3, nr 6, artikkel-id e1700345Artikkel i tidsskrift (Fagfellevurdert)
    Abstract [en]

    Poly(3,4-ethylenedioxythiophene): polystyrene sulfonate (PEDOT:PSS) is an organic mixed ion-electron conducting polymer. The PEDOT phase transports holes and is redox-active, whereas the PSS phase transports ions. When PEDOT is redox-switched between its semiconducting and conducting state, the electronic and optical properties of its bulk are controlled. Therefore, it is appealing to use this transition in electrochemical devices and to integrate those into large-scale circuits, such as display or memory matrices. Addressability and memory functionality of individual devices, within these matrices, are typically achieved by nonlinear current-voltage characteristics and bistability-functions that can potentially be offered by the semiconductor-conductor transition of redox polymers. However, low conductivity of the semiconducting state and poor bistability, due to self-discharge, make fast operation and memory retention impossible. We report that a ferroelectric polymer layer, coated along the counter electrode, can control the redox state of PEDOT. The polarization switching characteristics of the ferroelectric polymer, which take place as the coercive field is overcome, introduce desired nonlinearity and bistability in devices that maintain PEDOT in its highly conducting and fast-operating regime. Memory functionality and addressability are demonstrated in ferro-electrochromic display pixels and ferro-electrochemical transistors.

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  • 2.
    Jonsson, Amanda
    et al.
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Inal, Sahika
    Department of Bioelectronics, Ecole Nationale Supérieure des Mines, CMP-EMSE, MOC, Gardanne, France .
    Uguz, Ilke
    Department of Bioelectronics, Ecole Nationale Supérieure des Mines, CMP-EMSE, MOC, Gardanne, France .
    Williamson, Adam
    Aix Marseille Université, INS, Marseille, France; Inserm, UMR_S 1106, Marseille, France.
    Kergoat, Loig
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten. Aix Marseille Université, INS, Marseille, France; Inserm, UMR_S 1106, Marseille, France.
    Rivnay, Jonathan
    Department of Bioelectronics, Ecole Nationale Supérieure des Mines, CMP-EMSE, MOC, Gardanne, France .
    Khodagholy, Dion
    Department of Bioelectronics, Ecole Nationale Supérieure des Mines, CMP-EMSE, MOC, Gardanne, France .
    Berggren, Magnus
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Bernard, Christophe
    Aix Marseille Université, INS, Marseille, France; Inserm, UMR_S 1106, Marseille, France.
    Malliaras, George G
    Department of Bioelectronics, Ecole Nationale Supérieure des Mines, CMP-EMSE, MOC, Gardanne, France .
    Simon, Daniel T
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Bioelectronic neural pixel: Chemical stimulation and electrical sensing at the same site2016Inngår i: Proceedings of the National Academy of Sciences of the United States of America, ISSN 0027-8424, E-ISSN 1091-6490, Vol. 113, nr 34, s. 9440-9445Artikkel i tidsskrift (Fagfellevurdert)
    Abstract [en]

    Local control of neuronal activity is central to many therapeutic strategies aiming to treat neurological disorders. Arguably, the best solution would make use of endogenous highly localized and specialized regulatory mechanisms of neuronal activity, and an ideal therapeutic technology should sense activity and deliver endogenous molecules at the same site for the most efficient feedback regulation. Here, we address this challenge with an organic electronic multifunctional device that is capable of chemical stimulation and electrical sensing at the same site, at the single-cell scale. Conducting polymer electrodes recorded epileptiform discharges induced in mouse hippocampal preparation. The inhibitory neurotransmitter, γ-aminobutyric acid (GABA), was then actively delivered through the recording electrodes via organic electronic ion pump technology. GABA delivery stopped epileptiform activity, recorded simultaneously and colocally. This multifunctional “neural pixel” creates a range of opportunities, including implantable therapeutic devices with automated feedback, where locally recorded signals regulate local release of specific therapeutic agents.

    Fulltekst (pdf)
    fulltext
  • 3.
    Kergoat, Loig
    et al.
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Herlogsson, Lars
    Thin Film Elect AB, Sweden .
    Piro, Benoit
    University of Paris Diderot Sorbonne Paris Cite, France .
    Chau Pham, Minh
    University of Paris Diderot Sorbonne Paris Cite, France .
    Horowitz, Gilles
    Ecole Polytech, France .
    Crispin, Xavier
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Berggren, Magnus
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Tuning the threshold voltage in electrolyte-gated organic field-effect transistors2012Inngår i: Proceedings of the National Academy of Sciences of the United States of America, ISSN 0027-8424, E-ISSN 1091-6490, Vol. 109, nr 22, s. 8394-8399Artikkel i tidsskrift (Fagfellevurdert)
    Abstract [en]

    Low-voltage organic field-effect transistors (OFETs) promise for low power consumption logic circuits. To enhance the efficiency of the logic circuits, the control of the threshold voltage of the transistors are based on is crucial. We report the systematic control of the threshold voltage of electrolyte-gated OFETs by using various gate metals. The influence of the work function of the metal is investigated in metal-electrolyte-organic semiconductor diodes and electrolyte-gated OFETs. A good correlation is found between the flat-band potential and the threshold voltage. The possibility to tune the threshold voltage over half the potential range applied and to obtain depletion-like (positive threshold voltage) and enhancement (negative threshold voltage) transistors is of great interest when integrating these transistors in logic circuits. The combination of a depletion-like and enhancement transistor leads to a clear improvement of the noise margins in depleted-load unipolar inverters.

    Fulltekst (pdf)
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  • 4.
    Kergoat, Loig
    et al.
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Piro, Benoit
    University of Paris Diderot, France .
    Simon, Daniel
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Minh-Chau Pham; Noel, Vincent
    University of Paris Diderot, France .
    Berggren, Magnus
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Detection of Glutamate and Acetylcholine with Organic Electrochemical Transistors Based on Conducting Polymer/Platinum Nanoparticle Composites2014Inngår i: Advanced Materials, ISSN 0935-9648, E-ISSN 1521-4095, Vol. 26, nr 32, s. 5658-5664Artikkel i tidsskrift (Fagfellevurdert)
    Abstract [en]

    The aim of the study is to open a new scope for organic electrochemical transistors based on PEDOT:PSS, a material blend known for its stability and reliability. These devices can leverage molecular electrocatalysis by incorporating small amounts of nano-catalyst during the transistor manufacturing (spin coating). This methodology is very simple to implement using the know-how of nanochemistry and results in efficient enzymatic activity transduction, in this case utilizing choline oxidase and glutamate oxidase.

    Fulltekst (pdf)
    fulltext
  • 5.
    Kergoat, Loig
    et al.
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Piro, Benoît
    Université Paris Diderot, France.
    Berggren, Magnus
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Horowitz, Gilles
    Université Paris Diderot, France.
    Pham, Minh-Chau
    Université Paris Diderot, France.
    Advances in organic transistor-based biosensors: from organic electrochemical transistors to electrolyte-gated organic field-effect transistors.2012Inngår i: Analytical and Bioanalytical Chemistry, ISSN 1618-2642, E-ISSN 1618-2650, Vol. 402, nr 5, s. 1813-1826Artikkel, forskningsoversikt (Fagfellevurdert)
    Abstract [en]

    Organic electronics have, over the past two decades, developed into an exciting area of research and technology to replace classic inorganic semiconductors. Organic photovoltaics, light-emitting diodes, and thin-film transistors are already well developed and are currently being commercialized for a variety of applications. More recently, organic transistors have found new applications in the field of biosensors. The progress made in this direction is the topic of this review. Various configurations are presented, with their detection principle, and illustrated by examples from the literature.

  • 6.
    Kergoat, Loig
    et al.
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Piro, Benoît
    Université Paris Diderot, France.
    Berggren, Magnus
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Pham, Minh-Chau
    Université Paris Diderot, France.
    Yassar, Abderrahim
    Ecole Polytechnique, Palaiseau, France.
    Horowitz, Gilles
    Université Paris Diderot, France.
    DNA detection with a water-gated organic field-effect transistor2012Inngår i: Organic electronics, ISSN 1566-1199, E-ISSN 1878-5530, Vol. 13, nr 1, s. 1-6Artikkel i tidsskrift (Fagfellevurdert)
    Abstract [en]

    A DNA sensor based on a water-gated organic field-effect transistor is described. The semiconductor is poly [3-(5-carboxypentyl)thiophene-2,5-diyl] onto which DNA probes are covalently grafted via NHS/EDC chemistry. Clear changes in the output characteristic of the device are observed upon DNA immobilization and after DNA hybridization. Experimental data point out the importance of the electrolyte Debye length that can screen negative DNA charges and impede transduction. For this reason, deionized water was used in order to increase the Debye length up to several hundreds of nanometers. In this case, a decrease in the off current was observed upon hybridization, whereas no significant change occurred when using saline solutions.

  • 7.
    Mitraka, Evangelia
    et al.
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Kergoat, Loig
    Linköpings universitet, Institutionen för teknik och naturvetenskap. Linköpings universitet, Tekniska fakulteten.
    Ullah Khan, Zia
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Fabiano, Simone
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Douheret, O.
    University of Mons UMons, Belgium.
    Leclere, P.
    University of Mons UMons, Belgium.
    Nilsson, M.
    Acreo AB, Sweden.
    Andersson Ersman, P.
    Acreo AB, Sweden.
    Gustafsson, G.
    Acreo AB, Sweden.
    Lazzaroni, R.
    University of Mons UMons, Belgium.
    Berggren, Magnus
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Crispin, Xavier
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Solution processed liquid metal-conducting polymer hybrid thin films as electrochemical pH-threshold indicators2015Inngår i: Journal of Materials Chemistry C, ISSN 2050-7526, E-ISSN 2050-7534, Vol. 3, nr 29, s. 7604-7611Artikkel i tidsskrift (Fagfellevurdert)
    Abstract [en]

    A global and accurate mapping of the environment could be achieved if sensors and indicators are mass-produced at low cost. Printed electronics using polymeric (semi) conductors offer a platform for such sensor/indicator based circuits. Herein, we present the material concept for an electrochemical pH-threshold indicator based on a printable hybrid electrode which comprises a liquid metal alloy (GaInSn) embedded in a conducting polymer matrix (PEDOT). This hybrid electrode displays a large variation in open circuit potential versus pH in an electrochemical cell, which when connected to the gate of an electrochemical transistor leads to a dramatic change in the drain current in a narrow range of pH.

    Fulltekst (pdf)
    fulltext
  • 8.
    Sinno, Hiam
    et al.
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Kergoat, Loig
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Fabiano, Simone
    Linköpings universitet, Institutionen för teknik och naturvetenskap. Linköpings universitet, Tekniska högskolan.
    Crispin, Xavier
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Berggren, Magnus
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Engquist, Isak
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Bias stress effect in inverters based on polyelectrolyte-gated organic field effect transistors2013Manuskript (preprint) (Annet vitenskapelig)
    Abstract [en]

    Prolonged gate bias application causes undesirable operational instabilities in organic transistors involving threshold voltage shift and drain current degradation; an effect known as bias stress. In this paper, we report how this instability is manifested in inverter circuits based on polyelectrolytegated p-type organic field effect transistors (EGOFETs) operating at low voltage. We find that bias stress causes a significant, but recoverable, shift in inverter switching threshold voltage. Measurements with two different polyelectrolytes reveal significant differences in the stressing and recovery behaviour, which is ascribed to the distinct nature of the ion conductive groups in the polyelectrolyte. Moreover, we report a large influence of illumination on the recovery process for one of the polyelectrolytes but not for the other, which demonstrates the need to characterize bias stress behavior for each new materials combination.

  • 9.
    Toss, Henrik
    et al.
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Suspene, Clement
    University of Paris Diderot, France .
    Piro, Benoit
    University of Paris Diderot, France .
    Yassar, Abderrahim
    Ecole Polytechnique, Palaiseau, France.
    Crispin, Xavier
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Kergoat, Loig
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    Pham, Minh-Chau
    University of Paris Diderot, France .
    Berggren, Magnus
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska högskolan.
    On the mode of operation in electrolyte-gated thin film transistors based on different substituted polythiophenes2014Inngår i: Organic electronics, ISSN 1566-1199, E-ISSN 1878-5530, Vol. 15, nr 10, s. 2420-2427Artikkel i tidsskrift (Fagfellevurdert)
    Abstract [en]

    Organic Thin Film Transistors (OTFT), gated through an aqueous electrolyte, have extensively been studied as sensors in various applications. These water-gated devices are known to work both as electrochemical (Organic ElectroChemical Transistor - OECT) and field-effect (Organic Field-Effect Transistor - OFET) devices. To properly model and predict the response of water-gated OTFT sensors it is important to distinguish between the mechanism, field-effect or electrochemical, by which the transistor is modulated and thus how the gate signal can be affected by the analyte. In this present study we explore three organic polymer semiconductors, poly-(3-hexyl-thiophene) (P3HT), poly-(3-carboxypentyl-thiphene) (P3CPT) and a co-polymer P3HT-co-poly-(3-ethoxypentanoic acid-thiophene) (monomer ratio 1:6, P3HT-COOH15) in water-gated OTFT structures. We report a set of transistor characteristics, including standard output parameters, impedance spectroscopy and current transients, to investigate the origin of the mode of operation in these water-gated OTFTs. Impedance characteristics, including both frequency and voltage dependence, were recorded for capacitor stacks corresponding to the gate/electrolyte/semiconductor/source structure. It is shown that P3HT as well as P3HT-COOH15 both can function as semiconductors in water gated OTFT devices operating in field-effect mode. P3CPT on the other hand shows typical signs of electrochemical mode of operation. The -COOH side group has been suggested as a possible anchoring site for biorecognition elements in EGOFET sensors, rendering P3HT-COOH15 a possible candidate for such applications.

    Fulltekst (pdf)
    fulltext
  • 10.
    Tu, Deyu
    et al.
    Linköpings universitet, Institutionen för systemteknik, Informationskodning. Linköpings universitet, Tekniska fakulteten.
    Kergoat, Loïg
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten. Norrköping Sweden.
    Crispin, Xavier
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten. Norrköping Sweden.
    Berggren, Magnus
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten. Norrköping Sweden.
    Forchheimer, Robert
    Linköpings universitet, Institutionen för systemteknik, Informationskodning. Linköpings universitet, Tekniska fakulteten.
    Transient analysis of electrolyte-gated organic field effect transistors2012Inngår i: SPIE Proceedings Vol. 8478: Organic Field-Effect Transistors XI / [ed] Zhenan Bao; Iain McCulloch, 2012, Vol. 8478, s. 84780L-1-84780L-8Konferansepaper (Fagfellevurdert)
    Abstract [en]

    A terminal charge and capacitance model is developed for transient behavior simulation of electrolyte-gated organic field effect transistors (EGOFETs). Based on the Ward-Dutton partition scheme, the charge and capacitance model is derived from our drain current model reported previously. The transient drain current is expressed as the sum of the initial drain current and the charging current, which is written as the product of the partial differential of the terminal charges with respect to the terminal voltages and the differential of the terminal voltages upon time. The validity for this model is verified by experimental measurements.

    Fulltekst (pdf)
    fulltext
  • 11.
    Williamson, Adam
    et al.
    Aix Marseille University, France; INSERM, France.
    Rivnay, Jonathan
    Ecole National Super Mines, France.
    Kergoat, Loig
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Jonsson, Amanda
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Inal, Sahika
    Ecole National Super Mines, France.
    Uguz, Ilke
    Ecole National Super Mines, France.
    Ferro, Marc
    Ecole National Super Mines, France.
    Ivanov, Anton
    Aix Marseille University, France; INSERM, France.
    Arbring, Sjöström, Theresia
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Simon, Daniel
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Berggren, Magnus
    Linköpings universitet, Institutionen för teknik och naturvetenskap, Fysik och elektroteknik. Linköpings universitet, Tekniska fakulteten.
    Malliaras, George G.
    Ecole National Super Mines, France.
    Bernard, Christophe
    Aix Marseille University, France; INSERM, France.
    Controlling Epileptiform Activity with Organic Electronic Ion Pumps2015Inngår i: Advanced Materials, ISSN 0935-9648, E-ISSN 1521-4095, Vol. 27, nr 20, s. 3138-3144Artikkel i tidsskrift (Fagfellevurdert)
    Abstract [en]

    In treating epilepsy, the ideal solution is to act at a seizure's onset, but only in the affected regions of the brain. Here, an organic electronic ion pump is demonstrated, which directly delivers on-demand pure molecules to specific brain regions. State-of-the-art organic devices and classical pharmacology are combined to control pathological activity in vitro, and the results are verified with electrophysiological recordings.

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