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Formation of 3D Cr2C through solid state reaction-mediated Al extraction within Cr2AlC/Cu thin films
Rhein Westfal TH Aachen, Germany.
Linköping University, Department of Physics, Chemistry and Biology, Thin Film Physics. Linköping University, Faculty of Science & Engineering.ORCID iD: 0000-0003-3203-7935
Rhein Westfal TH Aachen, Germany.
Rhein Westfal TH Aachen, Germany.
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2025 (English)In: Nanoscale, ISSN 2040-3364, E-ISSN 2040-3372, Vol. 17, no 9, p. 5447-5455Article in journal (Refereed) Published
Abstract [en]

We report on the formation of the Cr2C compound using chemical etching-free methodology to extract Al from a Cr2AlC MAX phase thin film. Cr2AlC/Cu assemblies were deposited on sapphire substrates, using magnetron sputtering, and were subsequently annealed in vacuum. The Al from the MAX phase was shown to diffuse into Cu resulting in the formation of Al4Cu9 and causing the MAX phase to collapse into Cr2C grains. These carbide grains were characterized by transmission electron microscopy and the interatomic distances extracted were in good agreement with ab initio calculations predicting the equilibrium volume of the Cr2C phase.

Place, publisher, year, edition, pages
ROYAL SOC CHEMISTRY , 2025. Vol. 17, no 9, p. 5447-5455
National Category
Materials Chemistry
Identifiers
URN: urn:nbn:se:liu:diva-211604DOI: 10.1039/d4nr03664fISI: 001411400600001PubMedID: 39898885Scopus ID: 2-s2.0-85217202684OAI: oai:DiVA.org:liu-211604DiVA, id: diva2:1936717
Note

Funding Agencies|European Union; Swedish Research Council (VR); Swedish Foundation for Strategic Research (SSF); Swedish National Infrastructure in Advanced Electron Microscopy [2021-00171, RIF21-0026]; IT Center of RWTH Aachen University; Swedish Government Strategic Research Area in Materials Science on Functional Materials at Linkoeping University [2009 00971]; Knut and Alice Wallenberg foundation through the Wallenberg Academy Fellows program [KAW-2020.0196]; [892501]

Available from: 2025-02-11 Created: 2025-02-11 Last updated: 2026-03-06Bibliographically approved

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Palisaitis, JustinasPersson, PerEklund, Per

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