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Overcome Limited Efficiency in All-Perovskite Tandem Solar Cells Upon Light Management at Top Perovskite- Transparent Electrode Interfaces
Yangzhou Univ, Peoples R China.
Yangzhou Univ, Peoples R China.
Linköping University, Department of Science and Technology, Laboratory of Organic Electronics. Linköping University, Faculty of Science & Engineering.ORCID iD: 0000-0002-3190-2774
2025 (English)In: Advanced Electronic Materials, E-ISSN 2199-160X, Vol. 11, no 13, article id 2500019Article in journal (Refereed) Published
Abstract [en]

Tandem solar cells have gained significant attention due to their rapid advancements in power conversion efficiency (PCE) and their potential to exceed the detailed balance limit of single-junction solar cells. However, despite ongoing progress in perovskite-silicon tandem solar cells, all-perovskite tandem solar cells (APTSCs) still lag their perovskite-silicon counterparts. This raises the question: can further development close this gap? Upon theoretical modeling combining optical and electrical calculations, we found that: i) the PCE limitations in APTSCs are primarily caused by the reflection losses at the top perovskite interface; ii) introducing random texturing at the surfaces of wide-bandgap perovskites plays a critical role in enhancing light absorption, which can potentially improve PCE up to 30.97%. This improvement can be attributed to the reduced reflection and increased absorption at both the top wide-bandgap and the bottom narrow-bandgap perovskites. Furthermore, comparison between the calculated results and the experimental data clearly highlights the importance of light management strategies, particularly in improving the short-circuit current density. This approach is more effective than relying solely on interfacial passivation and energy band alignment to enhance the open-circuit voltage. The findings will provide valuable theoretical insights for optimizing and advancing the performance of APTSCs.

Place, publisher, year, edition, pages
WILEY , 2025. Vol. 11, no 13, article id 2500019
Keywords [en]
finite element method; light management; perovskite; tandem solar cells
National Category
Other Materials Engineering
Identifiers
URN: urn:nbn:se:liu:diva-213439DOI: 10.1002/aelm.202500019ISI: 001470359400001Scopus ID: 2-s2.0-105005180107OAI: oai:DiVA.org:liu-213439DiVA, id: diva2:1956330
Note

Funding Agencies|NSFC [62375234]; Science and Technology on Metrology and Calibration Laboratory [JLKG2024001C004, JLKG2023001C007]; Qing-Lan Project from Yangzhou University; Swedish Research Council [2022-04818]; Swedish Government Strategic Research Area in Materials Science on Functional Materials at Linkoeping University [2009 0097]

Available from: 2025-05-06 Created: 2025-05-06 Last updated: 2025-10-14Bibliographically approved

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Liu, Xianjie

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