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Towards rainbow photo/electro-luminescence in copper(i) complexes with the versatile bridged bis-pyridyl ancillary ligand
Normandie Univ, France; Univ Autonoma Madrid, Spain.
Technical University of Munich, Chair of Biogenic Functional Materials, Schulgasse 22, 94315 Straubing, Germany.
Normandie Univ, France; Tech Univ Munich, Germany.
Normandie Univ, France.
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2021 (English)In: Dalton Transactions, ISSN 1477-9226, E-ISSN 1477-9234, Vol. 50, no 32, p. 11049-11060Article in journal (Refereed) Published
Abstract [en]

The synthesis and characterization of a family of copper(i) complexes bearing a bridged bis-pyridyl ancillary ligand is reported, highlighting how the bridge nature impacts the photo- and electro-luminescent behaviours within the family. In particular, the phosphonium bridge led to copper(i) complexes featuring good electrochemical stability and high ionic conductivity, as well as a stark blue-to-orange luminescence shift compared to the others. This resulted in high performance light-emitting electrochemical cells reaching stabilities of 10 mJ at ca. 40 cd m(-2) that are one order of magnitude higher than those of the other complexes. Overall, this work sheds light onto the crucial role of the bridge nature of the bis-pyridyl ancillary ligand on the photophysical features, film forming and, in turn, on the final device performances.
Place, publisher, year, edition, pages
ROYAL SOC CHEMISTRY , 2021. Vol. 50, no 32, p. 11049-11060
National Category
Inorganic Chemistry
Identifiers
URN: urn:nbn:se:liu:diva-178477DOI: 10.1039/d1dt01689jISI: 000674899900001PubMedID: 34286773OAI: oai:DiVA.org:liu-178477DiVA, id: diva2:1587629
Note

Funding Agencies|Ministere de la Recherche et des Nouvelles Technologies; CNRS (Centre National de la Recherche Scientifique)Centre National de la Recherche Scientifique (CNRS); LABEX SynOrg [ANR-11-LABX-0029]; Region NormandieRegion Normandie; Normandie University; European UnionEuropean Commission [863170]; ERC-Co InOutBioLight [816856]; MSCA-ITN STiBNite [956923]; Spanish Ministerio de Ciencia, Innovacion y Universidades [RTI2018-097508-B-I00]; European UnionEuropean Commission; Comunidad de MadridComunidad de Madrid [S2018/NMT-4511]; "Severo Ochoa" Programme for Centres of Excellence in RD (MINECO) [SEV-2016-0686]; SeRC (Swedish e-Science Research Center)

Available from: 2021-08-25 Created: 2021-08-25 Last updated: 2021-09-02Bibliographically approved

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