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Chemical recycling to monomer: thermodynamic and kinetic control of the ring-closing depolymerization of aliphatic polyesters and polycarbonates
Wallenberg Wood Science Center, WWSC, Department of Fibre and Polymer Technology, KTH Royal Institute of Technology, Teknikringen 56-58, 100 44 Stockholm, Sweden.
Wallenberg Wood Science Center, WWSC, Department of Fibre and Polymer Technology, KTH Royal Institute of Technology, Teknikringen 56-58, 100 44 Stockholm, Sweden.ORCID iD: 0000-0002-5081-1835
Wallenberg Wood Science Center, WWSC, Department of Fibre and Polymer Technology, KTH Royal Institute of Technology, Teknikringen 56-58, 100 44 Stockholm, Sweden.ORCID iD: 0000-0002-7790-8987
Wallenberg Wood Science Center, WWSC, Department of Fibre and Polymer Technology, KTH Royal Institute of Technology, Teknikringen 56-58, 100 44 Stockholm, Sweden.ORCID iD: 0000-0002-5850-8873
2023 (English)In: Polymer Chemistry, ISSN 1759-9954, E-ISSN 1759-9962, Vol. 14, no 28, p. 3270-3276Article in journal (Refereed) Published
Abstract [en]

The thermodynamic equilibrium between ring-opening polymeriz[1]ation and ring-closing depolymerization is influenced by monomer–solvent–polymer interactions, an effect that can be uti[1]lized to promote chemical recycling to monomer. Here, the influence of monomer structure on this solvent effect has been investigated, showing that the chemical structure of the monomer influences the power of the solvent to supress the ceiling tempera[1]ture. The study also demonstrates how catalyst selectivity can be utilized to obtain selective ring-closing depolymerization of one component of a polymer blend, even when the thermodynamics dictate otherwise. 

Place, publisher, year, edition, pages
2023. Vol. 14, no 28, p. 3270-3276
National Category
Polymer Chemistry
Identifiers
URN: urn:nbn:se:liu:diva-207523DOI: 10.1039/d3py00535fOAI: oai:DiVA.org:liu-207523DiVA, id: diva2:1896640
Funder
Knut and Alice Wallenberg FoundationAvailable from: 2024-09-10 Created: 2024-09-10 Last updated: 2024-09-23

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